Introduction | p. 1 |
Optics of Nonlinear Crystals | p. 3 |
Three- and Four-Wave (Three- and Four-Frequency) Interactions in Nonlinear Media | p. 3 |
Phase-Matching Conditions | p. 5 |
Optics of Uniaxial Crystals | p. 6 |
Types of Phase Matching in Uniaxial Crystals | p. 10 |
Calculation of Phase-Matching Angles in Uniaxial Crystals | p. 13 |
Reflection and Refraction of Light Waves at the Surfaces of Uniaxial Crystals | p. 14 |
Optics of Biaxial Crystals | p. 16 |
Types of Phase Matching in Biaxial Crystals | p. 18 |
Calculation of Phase-Matching Angles in Biaxial Crystals | p. 19 |
Crystal Symmetry and Effective Nonlinearity: Uniaxial Crystals | p. 23 |
Crystal Symmetry and Effective Nonlinearity: Biaxial Crystals | p. 25 |
Theory of Nonlinear Frequency-Conversion Efficiency | p. 32 |
Wave Mismatch and Phase-Matching Bandwidth | p. 40 |
Calculation of Nonlinear Frequency-Conversion Efficiency in Some Special Cases | p. 48 |
Plane-Wave Fixed-Field Approximation | p. 49 |
Fundamental Wave Depletion ("Nonlinear Regime") | p. 52 |
SHG of a Divergent Fundamental Radiation Beam in the Fixed-Field Approximation | p. 54 |
SHG of a Divergent Fundamental Radiation Beam in the Nonlinear Regime | p. 55 |
Fixed-Intensity Approximation | p. 57 |
Frequency Conversion of Ultrashort Laser Pulses | p. 59 |
Frequency Conversion of Laser Beams with Limited Aperture in the Stationary Regime | p. 61 |
Linear Absorption | p. 65 |
Additional Comments | p. 65 |
Properties of Nonlinear Optical Crystals | p. 67 |
Basic Nonlinear Optical Crystals | p. 68 |
LiB3O5, Lithium Triborate (LBO) | p. 68 |
KH2PO4, Potassium Dihydrogen Phosphate (KDP) | p. 78 |
KD2PO4, Deuterated Potassium Dihydrogen Phosphate (DKDP) | p. 85 |
NH4H2PO4, Ammonium Dihydrogen Phosphate (ADP) | p. 90 |
ß-BaB2O4, Beta-Barium Borate (BBO) | p. 96 |
LiIO3, Lithium Iodate | p. 103 |
KTiOPO4, Potassium Titanyl Phosphate (KTP) | p. 107 |
LiNbO3, Lithium Niobate | p. 119 |
KNbO3, Potassium Niobate | p. 126 |
AgGaS2, Silver Thiogallate | p. 132 |
ZnGeP2, Zinc Germanium Phosphide | p. 136 |
Frequently Used Nonlinear Optical Crystals | p. 142 |
KB5O8 · 4H2O, Potassium Pentaborate Tetrahydrate (KB5) | p. 142 |
CO(NH2)2, Urea | p. 146 |
CsH2AsO4, Cesium Dihydrogen Arsenate (CDA) | p. 149 |
CsD2AsO4, Deuterated Cesium Dihydrogen Arsenate (DCDA) | p. 152 |
KTiOAsO4, Potassium Titanyl Arsenate (KTA) | p. 156 |
MgO : LiNbO3, Magnesium-Oxide-Doped Lithium Niobate | p. 159 |
Ag3AsS3, Proustite | p. 162 |
GaSe, Gallium Selenide | p. 166 |
AgGaSe2, Silver Gallium Selenide | p. 169 |
CdSe, Cadmium Selenide | p. 173 |
CdGeAs2, Cadmium Germanium Arsenide | p. 176 |
Other Inorganic Nonlinear Optical Crystals | p. 179 |
KB5O8 · 4D2O, Deuterated Potassium Pentaborate Tetrahydrate (DKB5) | p. 179 |
CsB3O5, Cesium Triborate (CBO) | p. 180 |
BeSO4 · 4H2O, Beryllium Sulfate | p. 182 |
MgBaF4, Magnesium Barium Fluoride | p. 184 |
NH4D2PO4, Deuterated Ammonium Dihydrogen Phosphate (DADP) | p. 186 |
RbH2PO4, Rubidium Dihydrogen Phosphate (RDP) | p. 188 |
RbD2PO4, Deuterated Rubidium Dihydrogen Phosphate (DRDP) | p. 192 |
KH2AsO4, Potassium Dihydrogen Arsenate (KDA) | p. 192 |
KD2AsO4, Deuterated Potassium Dihydrogen Arsenate (DKDA) | p. 195 |
NH4H2ASO4, Ammonium Dihydrogen Arsenate (ADA) | p. 196 |
NH4D2AsO4, Deuterated Ammonium Dihydrogen Arsenate (DADA) | p. 198 |
RbH2AsO4, Rubidium Dihydrogen Arsenate (RDA) | p. 199 |
RbD2AsO4, Deuterated Rubidium Dihydrogen Arsenate (DRDA) | p. 202 |
LiCOOH · H2O, Lithium Formate Monohydrate (LFM) | p. 204 |
NaCOOH, Sodium Formate | p. 207 |
Ba(COOH)2, Barium Formate | p. 209 |
Sr(COOH)2, Strontium Formate | p. 210 |
Sr(COO?)2 · 2H2O, Strontium Formate Dihydrate | p. 211 |
LiGaO2, Lithium Gallium Oxide | p. 213 |
¿-HIO3, ¿-Iodic Acid | p. 214 |
K2La(NO3)5 · 2H2O, Potassium Lanthanum Nitrate Dihydrate (KLN) | p. 217 |
CsTiOAsO4, Cesium Titanyl Arsenate (CTA) | p. 220 |
NaNO2, Sodium Nitrite | p. 221 |
Ba2NaNb5O15, Barium Sodium Niobate ("Banana") | p. 224 |
K2Ce(NO3)5 · 2H2O, Potassium Cerium Nitrate Dihydrate (KCN) | p. 227 |
K3Li2Nb5O15, Potassium Lithium Niobate | p. 229 |
HgGa2S4, Mercury Thiogallate | p. 231 |
HgS, Cinnibar | p. 233 |
Ag3SbS3, Pyrargyrite | p. 235 |
Se, Selenium | p. 236 |
Tl3AsS3, Thallium Arsenic Selenide (TAS) | p. 238 |
Te, Tellurium | p. 240 |
Other Organic Nonlinear Optical Crystals | p. 243 |
C12H22O11, Sucrose (Saccharose) | p. 243 |
L-Arginine Phosphate Monohydrate (LAP) | p. 245 |
Deuterated L-Arginine Phosphate Monohydrate (DLAP) | p. 247 |
L-Pyrrolidone-2-carboxylic Acid (L-PCA) | p. 250 |
CaC4H4O6 · 4H2O, Calcium Tartrate Tetrahydrate (L-CTT) | p. 251 |
(NH4)2C2O4 · H2O, Ammonium Oxalate (AO) | p. 253 |
m-Bis(aminomethyl)benzene (BAMB) | p. 254 |
3-Methoxy-4-hydroxy-benzaldehyde (MHBA) | p. 256 |
2-Furyl Methacrylic Anhydride (FMA) | p. 258 |
3-Methyl-4-nitropyridine-1-oxide (POM) | p. 259 |
Thienylchalcone (T-17) | p. 261 |
5-Nitrouracil (5NU) | p. 263 |
2-(N-Prolinol)-5-nitropyridine (PNP) | p. 265 |
2-Cyclooctylamino-5-nitropyridine (COANP) | p. 266 |
L-N-(5-Nitro-2-pyridyl) leucinol (NPLO) | p. 268 |
C6H4(NO2)2, m-Dinitrobenzene (MDNB) | p. 270 |
4-(N,N-Dimethylamino)-3-acetamidonitrobenzene (DAN) | p. 272 |
Methyl-(2,4-dinitrophenyl)-aminopropanoate (MAP) | p. 274 |
m-Nitroaniline (MNA) | p. 276 |
N-(4-Nitrophenyl)-N-methylaminoacetonitrile (NPAN) | p. 278 |
N-(4-Nitrophenyl)-L-prolinol (NPP) | p. 280 |
3-Methyl-4-methoxy-4'-nitrostilbene (MMONS) | p. 281 |
Properties of Crystalline Quartz (¿-SiO2) | p. 283 |
New Developments | p. 286 |
Applications of Nonlinear Crystals | p. 289 |
Generation of Neodymium Laser Harmonics | p. 289 |
Second-Harmonic Generation of Neodymium Laser Radiation in Inorganic Crystals | p. 289 |
Second-Harmonic Generation of 1,064 ¿m Radiation in Organic Crystals | p. 294 |
Intracavity SHG | p. 296 |
Third-Harmonic Generation | p. 298 |
Fourth-Harmonic Generation | p. 301 |
Fifth-Harmonic Generation | p. 301 |
Harmonic Generation of 1,318 ¿m Radiation | p. 304 |
Harmonic Generation of High-Power Large-Aperture Neodymium Glass Laser Radiation | p. 306 |
"Angle-Detuning" Scheme | p. 306 |
"Polarization-Mismatch" Scheme | p. 306 |
"Polarization-Bypass" Scheme | p. 308 |
Comparison of Schemes | p. 308 |
Experimental Results | p. 308 |
"Quadrature" Scheme | p. 310 |
Harmonic Generation for Other Laser Sources | p. 311 |
Ruby Laser | p. 311 |
Ti:sapphire Laser | p. 312 |
Semiconductor Lasers | p. 312 |
Dye Lasers | p. 315 |
Gas Lasers | p. 320 |
Iodine Laser | p. 321 |
CO2 Laser | p. 324 |
Other Lasers | p. 324 |
Frequency Conversion of Femtosecond Pulses | p. 326 |
Sum-Frequency Generation | p. 327 |
Up-Conversion to the UV Region | p. 328 |
Infrared Up-Conversion | p. 333 |
Up-Conversion of CO2 Laser Radiation to the Near IR and Visible Regions | p. 336 |
Difference Frequency Generation | p. 339 |
DFG in the Visible Region | p. 339 |
DFG in the Mid IR Region | p. 340 |
DFG in the Far IR Region | p. 344 |
Optical Parametric Oscillation | p. 345 |
OPO in the UV, Visible, and Near IR Spectral Regions | p. 345 |
OPO in the Mid IR Region | p. 359 |
Conversion of OPO Radiation to the UV Region | p. 360 |
Stimulated Raman Scattering and Picosecond Continuum Generation in Crystals | p. 362 |
References | p. 367 |
Appendix: List of Commonly Used Laser Wavelengths | p. 405 |
Subject Index | p. 407 |
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