Reaction Dynamics in Clusters and Condensed Phases

Proceedings of the Twenty-Sixth Jerusalem Symposium on Quantum Chemistry and Biochemistry held in Jerusalem, Israel, May 17-20, 1993

By: Joshua Jortner (Editor), R.D. Levine (Editor), A. Pullman (Editor)

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Hardcover | 31 December 1993

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The Twenty Sixth Jerusalem Symposium reflected the high standards of these distinguished scientific meetings, which convene once a year at the Israel Academy of Sciences and Humanities in Jerusalem to discuss a specific topic in the broad area of quantum chemistry and biochemistry. The topic at this year's Jerusalem Symposium was reaction dynamics in clusters and condensed phases, which constitutes a truly interdisciplinary subject of central interest in the areas of chemical dynamics, kinetics, photochemistry and condensed matter chemical physics. The main theme of the Symposium was built around the exploration of the interrelationship between the dynamics in large finite clusters and in infinite bulk systems. The main issues addressed microscopic and macroscopic sol vation phenomena, cluster and bulk spectroscopy, photodissociation and vibrational predissociation, cage effects, interphase dynamics, reaction dynamics and energy transfer in clusters, dense fluids, liquids, solids and biophysical systems. The interdisciplinary nature of this research area was deliberated by intensive and extensive interactions between modern theory and advanced experimental methods. This volume provides a record of the invited lectures at the Symposium.

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Preface
Elucidating the Influence of Solvations on the Dynamics of Cluster Reactions	p. 1
The Solvation of Halogen Anions in Water Clusters	p. 13
Excitation and Ionization of Chloride, Iodide, Bromide and Sodium in Water Clusters	p. 21
Photoelectron Spectroscopy of Solvated Anion Clusters	p. 37
Magic Numbers and Geminate Recombination Dynamics of Anions in Water Clusters	p. 47
Theoretical Spectroscopy and Dynamics of Tetra-Atomic Van der Waals Clusters	p. 57
Caging and Nonadiabatic Electronic Transitions in I[subscript 2]-M Complexes	p. 73
Phase Separation in Binary Clusters	p. 89
Molecular Collisions on Large Argon Clusters	p. 101
Spectra of Conformers of Mass Selected Van der Waals Clusters	p. 115
High Resolution IR Studies of Polymolecular Clusters : Micromatrices and Unimolecular Ring Opening	p. 137
Electronic Spectra of a Lithium Impurity in Clusters, the Bulk Liquid and Solid para-Hydrogen	p. 153
Localization of Electrons at Interfaces	p. 169
Solvation and Charge Transfer at Liquid Interfaces	p. 179
Second Harmonic and Sum Frequency Studies of Chemical Equilibria and Phase Transitions at Liquid Interfaces	p. 195
Isomerization Reactions at Aqueous Interfaces	p. 207
Ultrafast Solvation Dynamics by Degenerate Four Wave Mixing : a Theoretical and Experimental Study	p. 227
Femto-Second Photodissociation of Triiodide in Solution	p. 245
Solvent Polarity Effects on Cis-Stilbene Photochemistry from the First Femtoseconds to the Final Products	p. 261
Simulation of Electronic Spectroscopy and Relaxation in Aqueous Solution	p. 279
Electronic Structure and Chemical Reactions in Solution	p. 289
Suppression of Activated Rate Processes Induced by Space Dependent, Time Dependent and Anisotropic Friction	p. 311
Multidimensional Kramers and the Onset of Protein Relaxation	p. 331
Nonbinary Bimolecular Relaxation in Solutions	p. 343
Pressure Dependence of Solvent Effects in Elementary Reactions in Dense Media	p. 361
The Reorientational Dynamics in Liquid Methanol	p. 383
Molecular Theory of Vibrational Energy Relaxation in Gases and Liquids	p. 393
Quantum Mechanical Calculations of Tunneling Rates in Condensed Phase Systems	p. 411
How do the Properties of Water in Confined Volumes Differ from those in the Normal Liquid?	p. 423
Solvent Mean Force Perturbations of Molecular Vibration, Isomerization and Dissociation	p. 441
Molecular Theory of Optical Absorption Lineshapes of Dilute Solutes in Liquids : A Probe of Solvent Dynamics	p. 461
Multiple Time Scales in Molecular Dynamics : Applications to Vibrational Relaxation	p. 471
New Approaches to Solution Reaction Dynamics : Quantum Control and Ultrafast Diffraction	p. 495
Dynamics of the Cage Effect for Molecular Photodissociation in Solids	p. 509
Cage Effect and Molecular Dynamics of Cl[subscript 2] in Rare Gas Solids	p. 521
Electronic Energy Transfer in the Naphthalene-Anthracene Bichromophoric Molecular Cluster	p. 539
Electron Solvation : Quantum and Classical Aspects	p. 557
Table of Contents provided by Blackwell. All Rights Reserved.

Reaction Dynamics in Clusters and Condensed Phases

Proceedings of the Twenty-Sixth Jerusalem Symposium on Quantum Chemistry and Biochemistry held in Jerusalem, Israel, May 17-20, 1993

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